Researchers from University of Electronic Science and Technology of China (UESTC), CNRS, Guangzhou University and China Jiliang University have developed a slot-die coating strategy based on pyrrodiazole (PZ) additives in the perovskite precursor solution to simultaneously immobilize lead iodide and formamidinium iodide.
Image from: Nature Communications
This approach is meant to enhance wet film stability by suppressing colloidal aggregation, retards the crystal growth process, and ensures a consistent growth rate across the films. These effects can promote the formation of large, monolithic grains, enabling large-area perovskite films with homogeneous structure, excellent uniformity, and low defect density under ambient conditions. Using this strategy, the scientists achieved 10 cm × 10 cm inverted perovskite solar modules with a certified efficiency of 20.3% and retained 94% of initial efficiency after 1,000 h in standard testing, along with good working stability and excellent application demonstration, showcasing its great potential for industrialization.